Total gaseous mercury emissions from mercury-enriched soil in Guizhou, China     

Xinbin FENG Shaofeng WANG Guangle QIU Yamin HOU Shunlin TANG 《中国地球化学学报》2006,25(B08):243-244

Guizhou is located in the Circum-Pacific Global Mercuriferous Belt, and mercury concentrations in soil in this area are enriched. In-situ total gaseous mercury （TGM） exchange fluxes between air and soil surface were intensively measured at four sampling sites in Guiyang from 21 May to 16 June, 2003, and five sites in the Lanmuchang mercury mining area in December 2002 and May 2003, respectively. The in-situ Hg flux measurement was conducted with a dynamic flux chamber （DFC） of quartz. Overall, net emissions were obtained from all sampling sites. Soil mercury concentration and solar radiation have been proved to be the two most important parameters to control mercury emissions from soil. Meanwhile, rain events can enhance mercury emission rate significantly.  相似文献   

Palaeovariations in the East-Asian Monsoon Regime Geochemically Recorded in Varved Sediments of Lake Sihailongwan (Northeast China, Jilin Province). Part 2: a 200-Year Record of Atmospheric Lead-210 Flux Variations and its Palaeoclimatic Implications     

Georg Schettler  Jens Mingram  Jörg F. W. Negendank  Liu Jiaqi 《Journal of Paleolimnology》2006,35(2):271-288

Palaeovariations of the atmospheric ²¹⁰Pb flux in Northeast China (Long Gang area, Jilin province), quantified by high resolution ²¹⁰Pb measurements on seasonally laminated sediments of Lake Sihailongwan are presented on decadal scale. The mean flux of unsupported ²¹⁰Pb between 1790 and 1970 for the centre of the lake basin is 517 Bq m⁻² yr⁻¹ with maximum deviations between −23% and +27% of this value. Flux rates above this average were found between 1783 and 1813, around 1836, and between 1860 and 1901. The mean ²¹⁰Pb^exc flux rates derived were clearly lower around 1821, 1908, 1930, and 1953. The ²¹⁰Pb^exc flux reached its minimum of 344 Bq m⁻² yr⁻¹ during the period 1977–1982. The atmospheric flux of unsupported ²¹⁰Pb is correlated with the precipitation frequency during the summer monsoon and shows coinciding variability with geochemical proxies that document the groundwater inflow into the lake. Al₂O₃-rich dust of remote provenance scavenged by wet-deposition in the rainy season is the major carrier of the atmospheric ²¹⁰Pb^exc flux.  相似文献   

Palaeovariations in the East-Asian Monsoon Regime Geochemically Recorded in Varved Sediments of Lake Sihailongwan (Northeast China, Jilin Province). Part 1: Hydrological Conditions and Dust Flux   总被引：2，自引：0，他引：2  

Georg Schettler  Qiang Liu  Jens Mingram  Jörg F. W. Negendank 《Journal of Paleolimnology》2006,35(2):239-270

The varved sediments of the dimictic Lake Sihailongwan (Long Gang mountain area, Jilin Province, Northeast China) represent a palaeoclimatic archive which documents the local precipitation frequency during the summer monsoon, and variations in the aeolian flux of dust with their remote sources in the arid and semi-arid regions of inner Asia. Based on a detailed discussion of sediment genesis in Lake SHL, dust flux rates and palaeohydrological conditions were reconstructed on a decadal scale over the past 220 years. The aeolian influx by dry and wet deposition was quantified and characterised in its chemical composition. Photosynthetic production in the lake is positively correlated with the inflow of nutrient-rich groundwater. The groundwater discharge largely reflects the strength of the summer monsoon. Net accumulation rates for biogenic silica were determined for annually laminated sediments from the centre of the U-shaped lake basin based on sediment data. In a Si-balance model of the modern lake, the depositional flux of biogenic silica could be independently quantified on the base of hydrochemical monitoring data. Comparison of the both estimates allowed to asses the focussing of the particle flux in the lake. Though water retention in Lake SHL is rather high (ca. 30 years), changes in the hydrological conditions are sensitively recorded in the sediments because (i) nutrient-rich groundwater discharges into the productive zone of the lake, (ii) a substantial proportion of the total dissolved Si-inventory of the mixed lake (ca. 30%) is annually consumed by diatom growth, and (3) sediment accumulation is substantially focussed towards the flat bottom of the lake basin. The bulk siliciclastic sediment fraction (ca. 75 wt.%) largely originates from influx of dust of remote provenance. In sediment thin-sections, the dry-deposited dust fraction is microscopically identifiable as seasonal silt layer. Aeolian input by wet-deposition shows a distinctly higher variability than the influx of dust by dry-deposition. As diatom production, wet-deposition of dust is positively correlated with the rainfall during the summer monsoon. The inferred positive correlation between rainfall and dust flux during the summer monsoon implies that dust deposition is determined by the out-wash efficiency of mineral particles for a permanent high atmospheric dust concentration over Northeast China in the last 220 years.  相似文献   

粤北地区产铀岩体的铀矿化特征及其成矿机制探讨   总被引：7，自引：0，他引：7  

张敏  陈培荣  陈卫锋 《化工矿产地质》2006,28(1):9-14,26

粤北地区是中国花岗岩型铀矿最为重要的大型矿聚集区,其主要的产铀花岗岩体是诸广山岩体和贵东岩体,均为多期多阶段的复式岩体,主要以印支期和燕山期的花岗岩为主。粤北地区的铀矿床主要由诸广山的长江铀矿田、澜河铀矿田、鹿井铀矿田和贵东岩体的下庄铀矿田组成,根据铀的成矿特征可分为硅化带型、交点型和碱交代型。粤北地区的铀成矿流体主要来自于地幔,而不是以往认为的花岗岩浆期后热液,铀源主要是粤北产铀岩体的印支期花岗岩。因此在华南开展新一轮铀矿找矿时,跳出以往“沿带找矿”的老思路,聚焦于印支期岩浆作用与铀矿床的关系,并重点关注华南地区可能的地幔柱或热点区域。  相似文献   

大湾铀矿田铀-镭平衡系数及迁移富集特征研究     

刘红兵 《华南地质与矿产》2006,(1):34-37

从分析大湾铀矿田各矿床(点)的铀镭平衡系数变化特征出发,结合放射性同位素比值特征分析铀镭迁移富集行为,指出了各矿床(点)氧化带的深度,以了解各铀矿床(点)潜在的工业价值.  相似文献   

鄂尔多斯盆地北部底河道砂岩型铀矿地质特征   总被引：3，自引：0，他引：3  

吴仁贵  祝民强  余达淦  周万蓬 《华东地质学院学报》2006,29(1):1-6

鄂尔多斯盆地北部直罗组中的铀矿,是典型的产于河道中的砂岩铀矿,该矿床发育较好的卷状矿体。通过对该铀矿地质特征的研究,认识到发育卷状矿体的底河道砂岩型铀矿必须具备两大条件:其一是成矿砂体条件,即砂体要有较好的成层性、连通性和渗透性;其二是地层结构条件,即砂体必须存在较好的上、下隔水岩层。就砂体而言,河流相辫状沉积砂体是形成卷状矿体的主要砂体,并且以具有从辫状河向曲流河完整演化的辫状沉积砂体较好。砂体的上、下隔水岩层则有多种表现形式:下隔水层可由不透水的基岩或湖相沉积泥岩等构成;上隔水层由不透水的湖相泥岩、曲流沉积地层或岩浆岩等构成。在层间氧化作用过程上,存在纵横两个方向的氧化,即存在与河道方向一致的纵向氧化和与河道垂直的横向氧化,两种氧化作用成矿常叠加形成复杂的矿体类型;在矿化赋存的部位上,铀砂体通常发育在基底之上或不同建造之间;在古气候演变上,成矿作用发生在干旱气候条件下,或由潮湿向干旱的气候转变阶段。  相似文献   

胞外聚合物对膜生物反应器运行性能的影响   总被引：3，自引：1，他引：3  

张凤君  王顺义  邓锡斌  赵芝清  沙娜  王鹤 《吉林大学学报(地球科学版)》2006,(Z1)

膜生物反应器处理污水过程中,依据胞外聚合物(EPS)、蛋白质、多糖、粘度等参数随时间的变化趋势以及对膜通量的影响,求出上述参数及蛋白质/多糖的比值与膜通量间的相关系数分别为0.28、0.57、0.38、0.14、0.70。结果表明:蛋白质/多糖的比值与膜通量的衰减速度两者相关系数最大。  相似文献   

REE/trace element characteristics of sandstone-type uranium deposits in the Ordos Basin     

凌明星  杨晓勇  孙卫  苗建宇  刘池阳 《中国地球化学学报》2006,25(4):355-365

1 Introduction The Ordos Basin is the second largest sedimentary basin in China. During the last 10 years, a great progress has been achieved in the aspects of tectonic evolution, dynamics process, inner and outer geological processes during Mesozoic-Cen…  相似文献   

Application of membrane technology for water treatment： Ultrasound-associated cleaning of fouled microfiltration membranes     

Rui CHEN Xiaoli WANG Yonggang ZHANG Xueqi FU 《中国地球化学学报》2006,25(B08):128-129

The use of membranes is a widely employed, versatile, and effective separation process. One of the limiting aspects in applying microfiltration （MF） for wastewater treatment is that of problems with membrane fouling and consequent flux reduction. Membrane fouling occurs by the irreversible deposition of retained particles, colloids, macromolecules, salts, etc. at the membrane surface and/or inside the membrane. The predominant fouling mechanisms observed with MF membranes are classified as three categories： the build-up of a cake layer on the membrane surface, blocking of membrane pores, and adsorption of fouling material on the membrane surface or in the pore walls. Although many techniques have been developed to overcome fouling, studies on membrane cleaning still seem to be insufficient for practical membrane filtration systems. Current membrane cleaning technologies include hydraulic, chemical, and mechanical methods. Ultrasound （US） has been widely used as a method of cleaning materials because of the cavitation phenomenon. In this study, US cleaning technique was applied to removing the fouling of polyvinglidenefluoride （PVDF） MF membrane, which was used to treat yeast cell and isolated soybean protein （ISP） solution, respectively. The US employed 40 kHz frequency and the output power of 1.43-2.85 W/cm^2. The evolution of the cleaning effect is followed by the measurements of the flux recovery rate （FRstat） and the cleaning time cycle. Results showed that the membrane property, which was fouled by yeast cell solution, could be recovered by water cleaning with US irradiation. And the cleaning time with the same FRstat decreased with the increase of US intensity.  相似文献   

土壤天然热释光法在相山火山岩型铀矿床中的应用   总被引：1，自引：0，他引：1  

许军才  黄临平  刘庆成  董业才  魏海  龙期华 《物探与化探》2005,29(3):224-226

介绍了天然热释光法在火山岩铀矿床上的应用效果,表明矿体上方热释光异常较大,无矿区域异常较小,矿体的分布范围与高值异常范围一致,还发现在一些构造薄弱带,裂隙、断层处出现大的异常,试验证明土壤天然热释光测量可以为评价火山岩铀资源提供线索。  相似文献